You can contact Sophia Myles by writing through her agent. This is the address:
Sophia Myles
c/o Christian Hodell
Fifth Floor, 66-68 Margaret Street
London
W1W 8SR
United Kingdom
Note
Judging by the amount of visitors this site has I suppose Sophia Myles is getting more and more fanmail. Therefore, if you wish to receive an answer or an autograph make sure you send a self-adressed and sufficiently stamped envelope along. If you live outside of the UK make sure to enclose International Reply Coupons. For more help concerning writing a celebrity visit FanMail. I’m sure Sophia Myles is appreciating us following these guidelines 
I myself have written Sophia through her agent in London in November 2003. I also sent some pictures along, asking for her signature. On December 24, 2003 I received all of them plus an agency picture back. I was so happy! So, I know for sure, that the London address works… Good luck!
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